This paper presents a method for continuously optimizing the turn-on and turn-off angles of a switched reluctance generator (SRG) operating in single-pulse mode and connected to an asymmetric bridge converter. The optimal angles are defined as those that minimize total SRG loss while ensuring accurate tracking of the terminal voltage reference. The Pearson correlation coefficient between SRG loss and selected SRG variables was calculated, with the highest correlation found for the average value of all phase currents. Therefore, the average phase current was selected as the variable to be minimized in a perturb-and-observe (P&O) method used to determine the optimal turn-on angle at a given operating point. The turn-off angle was calculated to maintain the terminal voltage at its reference value. The method was validated using both a conventional SRG simulation model and an advanced model that accounts for mutual coupling, iron losses, and remanent magnetism, and was further verified experimentally on an 8/6 SRG rated at 1.1 kW under various load conditions, terminal voltages, and rotor speeds.