We carry out multi-fluid simulations to study the plasma dynamics, particle acceleration, and formation of potential dips and peaks during an arc discharge in a plasma chamber. The initial condition of the simulation corresponds to a stable arc discharge already formed to ionize the gas. We note that establishing an arc discharge requires a voltage of hundreds to thousands of volts to initiate the spark. A stable arc current can then be formed and maintained at a low voltage (e.g., 100 volts) with a current of a few to tens of amperes. The stable arc discharge is then used as the initial condition.
We use the external electric potential 100 volts, 300 volts or 500 volts as the simulation boundary condition. The externally imposed potential is a time-independent boundary condition and is used for solving the 1D electrostatic Poisson Equation by using the tridiagonal matrix algorithm. It is similar to the formation of a conducting channel (return stroke) in gas-discharge lamps or in the air before the occurrence of lightning. It should be noted that the kink/sausage modes with their 2-D structure cannot occur in the 1-D approximation. In the proposed model, the emitted electrons at the cathode surface could further lead to the two-stream instability.
3.1. The Governing Equations
The discharge and current flow are mostly oriented along this thin and elongated conducting tube. Hence, we simplify the key physical process into a one-dimensional problem, similar to the approach for the conducting channel associated with lightning [
14]. Under this approximation, we developed a one-dimensional multi-fluid simulation code along the
x-axis to study the formation of the electrostatic potential in the arc discharge. The governing equations are the Poisson’s equation in electrostatics
the continuity equation
the momentum equation
and the ideal gas law
where
e is the fundamental charge or
Coulomb,
vacuum permittivity, and
charge density. The subscript
indicates fluid species and can be electron (e) and proton (p), and the subscript “n” stands for “neutral”. The fluid quantities are number density
n, velocity
, pressure
p, charge
q, electric field
E, collision frequency for charge particles to neutral
and temperature
T. The real proton to electron mass ratio is used
. The diffusion of electron and ion velocities through viscosity will be included and discussed later.
In the simulation with complete energy equation, we found that the arc plasma can be quickly heated to much higher than 1 eV. However, the plasma can be partially converted to other part of the chamber, which lowers the plasma temperature. The radiation loss also reduces the plasma temperature. The temperature of the plasma in the region where current flows through is estimated to be
6000 K [
18]. The simulation initial condition at
t = 0 corresponds to the time when the arc discharge is formed, and the plasma is heated to
We consider that the heating of the arc plasma from electricity and the heat loss through radiation and convection reach equilibrium during the simulation and that the temperature also reaches equilibrium in the conducting channel, which likely leads to constant temperature for all species
.
We have tried different system length ranging from 2 to 50 mm, and the length can affect the stability of the simulation and the formation of electrostatic waves. In this paper, we present the results associated with the system length of 2 mm, 5 mm, 8mm, 10 mm, 20 mm, 30 mm, 40 mm, and 50 mm. The other normalization parameters are neutral number density , electric potential 1 volt, velocity m/s (velocity of 1 eV proton) and time . The numerical time step and grid spacing are and . The neutrals in the conducting tube are assumed to be heated from 300 K to 6000 K. With a constant pressure across the chamber, the density in the conducting channel will be reduced as one-twentieth of .
In the present simulation study, the effect of ionization and recombination is minor during the simulation time scale of tens of nanoseconds. The plasma only exists in the arc discharge region. The other initial parameters at
of our simulation are neutral density
charge densities
, boundary electric potential
, and velocities
The ionization ratio is chosen based on Saha ionization equation [
19,
20]. Since the ionization ratio is very small and the ionization effect is minor during the simulation time scale, the neutral density
can be regarded as being constant in the simulation.
The hydrogen gas is weakly ionized and contains dominant neutral gas H
2. The proton-neutral collisional frequency [
21,
22,
23] is given by
and the electron-neutral collisional frequency is given by
Here the proton-neutral collision cross-section is
and the electron-neutral collision cross-section
[
23]. Equation (6) gives that the electron-neutral collision frequency is on the order of
Hz. The term
in the momentum equation comes from the charge-neutral collision effect. Since the neutral fluid is affected mainly through the proton-neutral collisional effect, the proton-neutral collision frequency
is on the order of
Hz. Note here that the proton to neutral mass density ratio is
. The relation
gives that the neutral to proton collision frequency is
. As a result, the neutral-proton collision frequency is of the order of
Hz due to the high neutral density compared with the charged fluid. Hence, in the time scale of nanosecond, the neutral fluid can be regarded as being immobile during the simulation period since the only momentum source for neutral fluid is from neutral-ion collisions. On the other hand, the collision effect exerts a “slowing-down” or drag force on the charged fluids.
In a weakly ionized gas, the electron and proton density diffusion coefficients due to thermal motion and collisions between charged and neutral fluids, to first order in the density, can be estimated as [
24]
We obtain and for .
On the other hand, the coefficient associated with bulk viscosity without mass density for electron and proton fluids can be estimated as
where
is a dimensionless factor in the range of 10-100 due to that the bulk viscosity is usually 10-100 times higher than the shear viscosity with
. The bulk viscosity, used in the numerical simulation, is of the order of theoretical value.
At every time step, the density diffusion and velocity viscosity terms are applied to the charge density (
and
) and to the velocity (
and
) via a three-point smooth scheme based on the diffusion and viscosity coefficients, respectively. The smoothing scheme plays the role of dissipation and also reduces the steepening of the fluid, similar to the dissipation term in the Burger’s equation. The three-point smooth scheme is derived from the finite difference form of the diffusion equation
where
and
for density or
for velocity.
In the continuity equations, a bounded (closed) boundary condition is used, i.e., the momentum and velocity are zero at boundaries. However, the emission of electrons at the surface of LaB
6 slab can lead to the increase of the electron density just outside the LaB
6 slab. The electron emission rate due to heating of LaB
6 slab is set to 10-15 amps [
25].
3.2. Two Simulation Cases Without and with Emission of Thermionic Electrons (
In order to examine the effect of the thermionic electron emission from LaB6, we simulate two cases without LaB6 and with LaB6.
Figure 3(a)shows a simulation without LaB
6 slab in the cathode and a 100V electric potential is applied across the gas chamber
with
. For a comparison,
Figure 3(b) shows the simulation results with the same parameters as in
Figure 3(a), but a LaB
6 slab is applied in the cathode.
In
Figure 3(a), an electric potential
is applied across the cathode (
. Some electrons in the plasma chamber are attracted by the applied positive potential at
to form a potential dip around point B. The lower potential at the cathode tends to attract ions to the left region between
and point A. The ion density near
is lower than the electron density near B. This may be due to larger ion mass (lower electron mass) and hence slower (faster) moving speed.
It is interesting to point out the electric potential profile is similar to the potential distribution between the cathode and anode in
Figure 4 of the review paper by Anders [
9]. The potential drop between points B and C is the positive anode fall, while the potential drop between the origin and point A is the negative cathode fall.
In
Figure 3(b), a simulation with LaB
6 slab installed in the cathode and 100 V potential is applied in the 20 mm chamber (
) between cathode and anode. The neutral H
2 is filled with
, which is equivalent to the density of
. The thermionic electrons are emitted from LaB
6 surface and carry 10A current. In this case, a potential dip near the LaB
6 surface can reach more than 1000 volts. In the arc discharge, the two-stream instability occurs and leads to potential peaks of a few hundreds of volts. The theory of two-stream instability will be developed in the following simulation case.
In the simulation case shown in
Figure 4, the density and velocity distributions in the x-t plane show clearly the presence and growth of wavy patterns, which are caused by the electron-ion two-stream instability. This case shows a clear pattern of the electrostatic waves. The potential peak can reach nearly 11.4 kV at
, and the dip can reach about -0.6 kV (not shown). The wavy potential structure may last for a few nanoseconds and quickly fades away. The number of peaks and dips depends on the plasma density and electron velocity. These waves are nearly stationary oscillations in plasma (electron) frame and can move in the laboratory frame.
The electron-ion two-stream instability can be solved by the linear plasma dispersion relation
where
is the electron plasma frequency,
the proton plasma frequency and
the wave number [
26,
27,
28,
29]. Here
is the wave frequency. The linear dispersion relation is solved based on the electrostatic two-fluid equations for cold and homogeneous plasmas. Note that the plasma frequency is on the order of
Hz, about one order of magnitude higher than the electron-neutral collision frequency. Hence, the collision effect can be ignored when solving this dispersion relation. As shown in
Figure 4, there is a long channel tube, in which the wave structure can be analyzed by the Fourier analysis of
and
k. The solution of
with nonzero wave growth rate
gives (a) the wave frequency
and (b) the wave number
The maximum wave growth rate
occurs at
and
as shown in
Figure 5. The corresponding wavelength can be expressed as
Based on the plasma parameters (
m/s,
, and
) and the linear theory, we obtain
and the maximum growth rate
from (11). For the simulation in
Figure 4, there are four potential peaks and the corresponding wavelength is
, close to the theoretical value
In
Figure 6(a), we plot the electric potential as a function of x at different simulation times,
t = 0.9, 1.0, …, 1.2 ns. It can be seen that the magnitude of electric potential peak and dip grows with time t for all four wave peaks and dips.
The growth rate of electric potential Peak 2 can be calculated from electron density peak values at different times. The growth rate of peaks is plotted as a function of time in
Figure 6(b). The growth rate of wave Peak 2 ranges from
to
, which is smaller than the maximum theoretical growth rate. This difference may be caused by the non-uniform profile of
and difference between simulated wavelength
and theoretical peak wavelength
.
In
Figure 7, we show the simulation (Case B in
Figure 3(b)) results at time
0.9, 1.0, 1.1, and 1.2 ns. In this case, an electric potential dip is formed due to the high-density electron layer and the magnitude can reach one kilovolt as shown in the electric potential profiles.
Thermionic emitted electrons lead to the formation of an electron layer near the left boundary (). As a result of this electron layer, the electric potential has a sharp decrease from to . The electric potential then increase gradually to volts at the right boundary (anode). The potential difference between and at is large. The average electric field in the chamber is negative (). The negative electric field in the chamber will accelerate electrons to high speed m/s, while ions are accelerated in the left direction with small velocity due to their large mass. The electrons and ions are accelerated in the opposite directions, which can lead to the electron-ion two-stream instability. In the electric potential profile, large amplitude electrostatic waves are formed due to this instability, and the wave amplitude may reach tens of kilovolts. The electron and ion number density and velocity profiles also show similar patterns. The wavy potential structure may last for a few ns.
In
Figure 7, the peak electric potential can reach about 2000V, the electric potential dip can reach -6.0 kV. Note that, in a weakly ionized plasma with temperature
0.5-0.75 eV, an electron can attach to a hydrogen atom H to form a negative hydrogen particle
. The density of negative hydrogen (
) is expected to be small compared with
density due to its low production rate [
30]. We ignore the contribution from
ions in the multi-fluid simulation. The formation of negative electric potential dips (positive electric potential peaks) can accelerate negative hydrogen ions (positive protons) toward the LaB
6 slab.
We estimate the diameter of the arc discharge by comparing a power input of 200 watts for the arc charge with the total kinetic and electric energy in the simulation domain. We calculate the total kinetic energy (electric energy) per area at
1.8 ns of the entire simulation domain and obtain 150
(164
). The energy provided by the power input at 200 watts over the period of 1.8 ns is
. We obtain an upper bound for the diameter
of the arc discharge
Note that the length of the arc discharge is 2 mm, which is 10 times of . Moreover, we also simulate cases of emitted thermionic current as 15A for three different sets of hydrogen pressure, three sets of applied voltage, and three sets of distances in the next section.
3.3. Comparisons for Simulation Results with Different Parameters
Table 1 lists 48 cases simulated with different set of parameters, which include the neutral H
2 pressure p, the neutral density
, the electric potential
at the anode, and the system (tube) length
. The resulting potential peak
and potential dip
are also listed in
Table 1.
Figure 8 shows the resulting
and
as a function of
(distance between cathode and anode) under applied voltages of 100V, 300V, and 500V from left to right columns. The top(bottom) panels in
Figure 8 show the resulting
. The red hollow circles are for the cases with 1 torr of neutral hydrogen pressure in the chamber. The black(blue) hollow circles denote the cases with 5torr (10torr) of neutral hydrogen (H
2) in the chamber. The resulting
ranges from 0.1 kV to 45.0 kV, while the resulting
ranges from 0.6 kV to 38.0 kV.
Table 1 and
Figure 8 show that Case 47 has the largest potential peak
). The largest potential dip is
in Case 47. In Case 47,
.
Figure 8 shows that the twenty-four cases with 1 torr have quasi-proportional value of
and of
with applied voltage
.
Regarding the dependence on (distance between cathode and anode), a larger has a larger with the same filling H2 pressure, while the dependence of is mixing.
Figure 9 shows the simulation results of Case 47 at
2.0 ns, 2.2 ns, 2.4 ns, and 2.6 ns. In this case, an electric potential dip is formed due to the high-density electron layer and the magnitude can reach -15.0 kV as shown in the electric potential profiles.
Thermionic emitted electrons lead to the formation of an electron layer near the left boundary (). As a result of this electron layer, the electric potential has a sharp decrease from to . The electric potential then increase gradually to volts at the right boundary (anode). The average electric field in the chamber is negative (). This negative average electric field in the chamber will accelerate electrons to high speed m/s, while ions are accelerated in the left direction with small velocity due to their large mass. The electrons and ions are accelerated in the opposite directions, which can lead to the electron-ion two-stream instability as discussed earlier. In the electric potential profile, large amplitude electrostatic waves are formed due to this instability, and the wave amplitude may reach tens of kilovolts. The electron and ion number density and velocity profiles also show similar patterns. The wavy potential structure may last for a few ns.