Submitted:
11 March 2025
Posted:
13 March 2025
You are already at the latest version
Abstract
The demand for computing power has been growing exponentially with the rise of artificial intelligence (AI), machine learning, and the Internet of Things (IoT). This growth requires unconventional computing primitives that prioritize energy efficiency, while also addressing the critical need for scalability. Neuromorphic computing, inspired by the biological brain, offers a transformative paradigm for addressing these challenges. This review paper provides an overview of advancements in 2D spintronics and device architectures designed for neuromorphic applications, with a focus on techniques such as spin-orbit torque, magnetic tunnel junctions, and skyrmions. Emerging van der Waals materials like CrI3, Fe3GaTe2, and graphene-based heterostructures have demonstrated unparalleled potential for integrating memory and logic at the atomic scale. This work highlights technologies with ultra-low energy consumption (0.14 fJ/operation), high switching speeds (sub-nanosecond), and scalability to sub-20 nm footprints. It covers key material innovations and the role of spintronic effects in enabling compact, energy-efficient neuromorphic systems, providing a foundation for advancing scalable, next-generation computing architectures.
Keywords:
1. Introduction
2. Fundamentals of Neuromorphic Computing
3. Overview of 2D Spintronic Materials
4. Spintronic Device Architectures for Neuromorphic Computing
4.1. MTJs and Spin Valves
4.2. Skyrmion-Based Devices
5. Scalability and Energy Efficiency
6. Applications in Neuromorphic Computing
7. Challenges and Future Outlooks
Author Contributions
Funding
Acknowledgments
Conflicts of Interest
References
- Chen, X.; Wang, L.; Wu, Y.; Gao, H.; Wu, Y.; Qin, G.; Wu, Z.; Han, Y.; Xu, S.; Han, T.; et al. Probing the electronic states and impurity effects in black phosphorus vertical heterostructures. 2D Materials 2016, 3, 015012. [Google Scholar] [CrossRef]
- Wu, Y.; Yin, G.; Pan, L.; Grutter, A.J.; Pan, Q.; Lee, A.; Gilbert, D.A.; Borchers, J.A.; Ratcliff, W.; Li, A.; et al. Large exchange splitting in monolayer graphene magnetized by an antiferromagnet. Nature Electronics 2020, 3, 604–611. [Google Scholar] [CrossRef]
- Wu, Y.; He, J.J.; Han, T.; Xu, S.; Wu, Z.; Lin, J.; Zhang, T.; He, Y.; Wang, N. Induced Ising spin-orbit interaction in metallic thin films on monolayer WSe2. Physical Review B 2019, 99, 121406. [Google Scholar] [CrossRef]
- Han, T.; Shen, J.; Yuan, N.F.; Lin, J.; Wu, Z.; Wu, Y.; Xu, S.; An, L.; Long, G.; Wang, Y.; et al. Investigation of the two-gap superconductivity in a few-layer NbSe2-graphene heterojunction. Physical Review B 2018, 97, 060505. [Google Scholar] [CrossRef]
- Gong, C.; Li, L.; Li, Z.; Ji, H.; Stern, A.; Xia, Y.; Cao, T.; Bao, W.; Wang, C.; Wang, Y.; et al. Discovery of intrinsic ferromagnetism in two-dimensional van der Waals crystals. Nature 2017, 546, 265–269. [Google Scholar] [CrossRef]
- Cao, G.; Meng, P.; Chen, J.; Liu, H.; Bian, R.; Zhu, C.; Liu, F.; Liu, Z. 2D Material Based Synaptic Devices for Neuromorphic Computing. Advanced Functional Materials 2021, 31, 2005443. [Google Scholar] [CrossRef]
- Wang, C.Y.; Wang, C.; Meng, F.; Wang, P.; Wang, S.; Liang, S.J.; Miao, F. 2D Layered Materials for Memristive and Neuromorphic Applications. Advanced Electronic Materials 2020, 6, 1901107. [Google Scholar] [CrossRef]
- Zhang, Z.; Yang, D.; Li, H.; Li, C.; Wang, Z.; Sun, L.; Yang, H. 2D materials and van der Waals heterojunctions for neuromorphic computing. Neuromorphic Computing and Engineering 2022, 2, 032004. [Google Scholar] [CrossRef]
- Yao, Y.; Cheng, H.; Zhang, B.; Yin, J.; Zhu, D.; Cai, W.; Li, S.; Zhao, W. Tunneling magnetoresistance materials and devices for neuromorphic computing. Materials Futures 2023, 2, 032302. [Google Scholar] [CrossRef]
- Chen, M.C.; Sengupta, A.; Roy, K. Magnetic Skyrmion as a Spintronic Deep Learning Spiking Neuron Processor. IEEE Transactions on Magnetics 2018, 54, 1–7. [Google Scholar] [CrossRef]
- Ma, Y.; Chen, M.; Aguirre, F.; Yan, Y.; Pazos, S.; Liu, C.; Wang, H.; Yang, T.; Wang, B.; Gong, C.; et al. Van der Waals Engineering of One-Transistor-One-Ferroelectric-Memristor Architecture for an Energy-Efficient Neuromorphic Array. Nano Letters 2025, 25, 2528–2537. [Google Scholar] [CrossRef] [PubMed]
- Rehman, M.M.; Samad, Y.A.; Gul, J.Z.; Saqib, M.; Khan, M.; Shaukat, R.A.; Chang, R.; Shi, Y.; Kim, W.Y. 2D materials-memristive devices nexus: From status quo to Impending applications. Progress in Materials Science 2025, 152, 101471. [Google Scholar] [CrossRef]
- Hadke, S.; Kang, M.A.; Sangwan, V.K.; Hersam, M.C. Two-Dimensional Materials for Brain-Inspired Computing Hardware. Chemical Reviews 2025, 125, 835–932. [Google Scholar] [CrossRef] [PubMed]
- Li, S.; Zhang, Z.; Mao, R.; Xiao, J.; Chang, L.; Zhou, J. A fast and energy-efficient SNN processor with adaptive clock/event-driven computation scheme and online learning. IEEE Transactions on Circuits and Systems I: Regular Papers 2021, 68, 1543–1552. [Google Scholar] [CrossRef]
- Yang, S.; Shin, J.; Kim, T.; Moon, K.W.; Kim, J.; Jang, G.; Hyeon, D.S.; Yang, J.; Hwang, C.; Jeong, Y.; et al. Integrated neuromorphic computing networks by artificial spin synapses and spin neurons. NPG Asia Materials 2021, 13, 11. [Google Scholar] [CrossRef]
- Zhou, J.; Chen, J. Prospect of Spintronics in Neuromorphic Computing. Advanced Electronic Materials 2021, 7, 2100465. [Google Scholar] [CrossRef]
- Sosa, L.; Wi, M.; Barrera, M.; Nasrullah, I.; Wu, Y. Simulating Pattern Recognition Using Non-volatile Synapses: MRAM, Ferroelectrics and Magnetic Skyrmions. arXiv 2025, arXiv:2501.03450. [Google Scholar]
- Chen, B.; Zeng, M.; Khoo, K.H.; Das, D.; Fong, X.; Fukami, S.; Li, S.; Zhao, W.; Parkin, S.S.; Piramanayagam, S.; et al. Spintronic devices for high-density memory and neuromorphic computing – A review. Materials Today 2023, 70, 193–217. [Google Scholar] [CrossRef]
- Lin, X.; Yang, W.; Wang, K.L.; Zhao, W. Two-dimensional spintronics for low-power electronics. Nature Electronics 2019, 2, 274–283. [Google Scholar] [CrossRef]
- Zhong, H.; Plummer, D.Z.; Lu, P.; Li, Y.; Leger, P.; Wu, Y. Integrating 2D magnets for quantum devices: from materials and characterization to future technology. Materials for Quantum Technology 2024, 5, 012001. [Google Scholar] [CrossRef]
- Zhang, B.; Lu, P.; Tabrizian, R.; Feng, P.X.L.; Wu, Y. 2D Magnetic heterostructures: spintronics and quantum future. Npj Spintronics 2024, 2, 6. [Google Scholar] [CrossRef]
- Verma, G.; Nisar, A.; Dhull, S.; Kaushik, B.K. Neuromorphic accelerator for spiking neural network using SOT-MRAM crossbar array. IEEE Transactions on Electron Devices 2023, 70, 6012–6020. [Google Scholar] [CrossRef]
- Verma, G.; Soni, S.; Nisar, A.; Kaushik, B.K. Multi-bit MRAM based high performance neuromorphic accelerator for image classification. Neuromorphic Computing and Engineering 2024, 4, 014008. [Google Scholar] [CrossRef]
- Wu, H.; Zhang, W.; Yang, L.; Wang, J.; Li, J.; Li, L.; Gao, Y.; Zhang, L.; Du, J.; Shu, H.; et al. Strong intrinsic room-temperature ferromagnetism in freestanding non-van der Waals ultrathin 2D crystals. Nature Communications 2021, 12, 5688. [Google Scholar] [CrossRef] [PubMed]
- Liu, R.; Liu, T.; Liu, W.; Luo, B.; Li, Y.; Fan, X.; Zhang, X.; Cui, W.; Teng, Y. SemiSynBio: A new era for neuromorphic computing. Synthetic and Systems Biotechnology 2024, 9, 594–599. [Google Scholar] [CrossRef] [PubMed]
- Wu, Y.; Sofer, Z.; Karuppasamy, M.; Wang, W. Room-temperature Ferroelectric Control of 2D Layered Magnetism. IEEE Transactions on Magnetics 2024, 1. [Google Scholar]
- Zhang, G.; Guo, F.; Wu, H.; Wen, X.; Yang, L.; Jin, W.; Zhang, W.; Chang, H. Above-room-temperature strong intrinsic ferromagnetism in 2D van der Waals Fe3GaTe2 with large perpendicular magnetic anisotropy. Nature Communications 2022, 13, 5067. [Google Scholar] [CrossRef] [PubMed]
- Burch, K.S.; Mandrus, D.; Park, J.G. Magnetism in two-dimensional van der Waals materials. Nature 2018, 563, 47–52. [Google Scholar] [CrossRef] [PubMed]
- Bonilla, M.; Kolekar, S.; Ma, Y.; Diaz, H.C.; Kalappattil, V.; Das, R.; Eggers, T.; Gutierrez, H.R.; Phan, M.H.; Batzill, M. Strong room-temperature ferromagnetism in VSe2 monolayers on van der Waals substrates. Nature Nanotechnology 2018, 13, 289–293. [Google Scholar] [CrossRef] [PubMed]
- Leger, P.A.; Ramesh, A.; Ulloa, T.; Wu, Y. Machine learning enabled fast optical identification and characterization of 2D materials. Scientific Reports 2024, 14, 27808. [Google Scholar] [CrossRef]
- Zhang, W.; Wong, P.K.J.; Zhu, R.; Wee, A.T.S. Van der Waals magnets: Wonder building blocks for two-dimensional spintronics? InfoMat 2019, 1, 479–495. [Google Scholar] [CrossRef]
- Wang, K.L.; Wu, Y.; Eckberg, C.; Yin, G.; Pan, Q. Topological quantum materials. MRS Bulletin 2020, 45, 373–379. [Google Scholar] [CrossRef]
- Vilà, M.; Hsu, C.; Garcia, J.H.; Benítez, L.A.; Waintal, X.; Valenzuela, S.O.; Pereira, V.M.; Roche, S. Low-symmetry topological materials for large charge-to-spin interconversion: The case of transition metal dichalcogenide monolayers. Physical Review Research 2020, 3, 043230. [Google Scholar] [CrossRef]
- Yasuda, K.; Tsukazaki, A.; Yoshimi, R.; Kondou, K.; Takahashi, K.; Takahashi, K.; Otani, Y.; Kawasaki, M.; Kawasaki, M.; et al. Current-Nonlinear Hall Effect and Spin-Orbit Torque Magnetization Switching in a Magnetic Topological Insulator. Physical Review Letters 2016, 119, 137204. [Google Scholar]
- Binda, F.; Avci, C.O.; Alvarado, S.F.; Noël, P.; Lambert, C.H.; Gambardella, P. Spin-orbit torques and magnetotransport properties of α-Sn and β-Sn heterostructures. Phys. Rev. B 2021, 103, 224428. [Google Scholar] [CrossRef]
- Wang, Y.; Deorani, P.; Banerjee, K.; Koirala, N.; Brahlek, M.J.; Oh, S.; Yang, H. Topological Surface States Originated Spin-Orbit Torques in Bi2Se3. Physical Review Letters 2015, 114 25, 257202. [Google Scholar]
- Singh, D.K.; Gupta, G. Brain-inspired computing: can 2D materials bridge the gap between biological and artificial neural networks? Materials Advances 2024, 5, 3158–3172. [Google Scholar] [CrossRef]
- Merkel, C.E. Synaptic Scaling and Optimal Bias Adjustments for Power Reduction in Neuromorphic Systems. 2023 IEEE 66th International Midwest Symposium on Circuits and Systems (MWSCAS); 2023; pp. 748–752. [Google Scholar]
- Gupta, S.; Vadde, V.; Muralidharan, B.; of Electrical Engineering, A.S.D.; of Technology Bombay, I.I.; Powai.; Mumbai-400076.; India.; of Engineering, D.S.S.A.C.; of Technology Ropar, I.I.; et al. A Comprehensive Convolutional Neural Network Architecture Design using Magnetic Skyrmion and Domain Wall. arXiv 2024, arXiv:2407.08469. [Google Scholar]
- Wu, Y.; Zhang, S.; Zhang, J.; Wang, W.; Zhu, Y.L.; Hu, J.; Yin, G.; Wong, K.; Fang, C.; Wan, C.; et al. Néel-type skyrmion in WTe2/Fe3GeTe2 van der Waals heterostructure. Nature Communications 2020, 11, 3860. [Google Scholar] [PubMed]
- Marfoua, B.; Hong, J. Highly efficient spin-orbit torque generation in bilayer WTe2/Fe3GaTe2 heterostructure. Materials Today Physics 2024, 42, 101378. [Google Scholar]
- Shin, I.; Cho, W.J.; An, E.S.; Park, S.; Jeong, H.W.; Jang, S.; Baek, W.J.; Park, S.Y.; Yang, D.H.; Seo, J.H.; et al. Spin–Orbit Torque Switching in an All-Van der Waals Heterostructure. Advanced Materials 2022, 34, 2101730. [Google Scholar] [CrossRef]
- Wang, H.; Wu, H.; Zhang, J.; Liu, Y.; Chen, D.; Pandey, C.; Yin, J.; Wei, D.; Lei, N.; Shi, S.; et al. Room temperature energy-efficient spin-orbit torque switching in two-dimensional van der Waals Fe3GeTe2 induced by topological insulators. Nature Communications 2023, 14, 5173. [Google Scholar] [PubMed]
- Mathon, J.; Umerski, A. Theory of tunneling magnetoresistance in a disordered Fe/MgO/Fe(001) junction. Physical Review B 2006, 74, 140404. [Google Scholar] [CrossRef]
- Jia, X.; Xia, K.; Bauer, G.E.W. Thermal Spin Transfer in Fe-MgO-Fe Tunnel Junctions. Physical Review Letters 2011, 107, 176603. [Google Scholar] [CrossRef]
- Li, X.; Lu, J.T.; Zhang, J.; You, L.; Su, Y.; Tsymbal, E.Y. Spin-dependent transport in van der Waals magnetic tunnel junctions with Fe3GeTe2 electrodes. Nano Letters 2019, 19, 5133–5139. [Google Scholar] [CrossRef] [PubMed]
- Li, D. Large magnetoresistance and efficient spin injection in ferromagnet/graphene/Fe3GeTe2 van der Waals magnetic tunnel junctions. The Journal of Physical Chemistry C 2021, 125, 16228–16234. [Google Scholar] [CrossRef]
- Zhang, L.; Li, T.; Li, J.; Jiang, Y.; Yuan, J.; Li, H. Perfect spin filtering effect on Fe3GeTe2-based van der Waals magnetic tunnel junctions. The Journal of Physical Chemistry C 2020, 124, 27429–27435. [Google Scholar] [CrossRef]
- Li, X.; Zhu, M.; Wang, Y.; Zheng, F.; Dong, J.; Zhou, Y.; You, L.; Zhang, J. Tremendous tunneling magnetoresistance effects based on van der Waals room-temperature ferromagnet Fe3GaTe2 with highly spin-polarized Fermi surfaces. Applied Physics Letters 2023, 122. [Google Scholar] [CrossRef]
- Tehrani, S.; Slaughter, J.; Deherrera, M.; Engel, B.; Rizzo, N.; Salter, J.; Durlam, M.; Dave, R.; Janesky, J.; Butcher, B.; et al. Magnetoresistive random access memory using magnetic tunnel junctions. Proceedings of the IEEE 2003, 91, 703–714. [Google Scholar] [CrossRef]
- Hu, J.M.; Li, Z.; Chen, L.Q.; Nan, C.W. High-density magnetoresistive random access memory operating at ultralow voltage at room temperature. Nature Communications 2011, 2, 553. [Google Scholar] [CrossRef] [PubMed]
- Cao, Q.; Lü, W.; Wang, X.R.; Guan, X.; Wang, L.; Yan, S.; Wu, T.; Wang, X. Nonvolatile Multistates Memories for High-Density Data Storage. ACS Applied Materials & Interfaces 2020, 12, 42449–42471. [Google Scholar] [CrossRef] [PubMed]
- Indiveri, G.; Chicca, E.; Douglas, R. A VLSI array of low-power spiking neurons and bistable synapses with spike-timing dependent plasticity. IEEE Transactions on Neural Networks 2006, 17, 211–221. [Google Scholar] [CrossRef] [PubMed]
- Younis, M.; Abdullah, M.; Dai, S.; Iqbal, M.A.; Tang, W.; Sohail, M.T.; Atiq, S.; Chang, H.; Zeng, Y.J. Magnetoresistance in 2D Magnetic Materials: From Fundamentals to Applications. Advanced Functional Materials 2025, 2417282. [Google Scholar] [CrossRef]
- Lim, C.K.; Devolder, T.; Chappert, C.; Grollier, J.; Cros, V.; Vaurès, A.; Fert, A.; Faini, G. Domain wall displacement induced by subnanosecond pulsed current. Applied Physics Letters 2004, 84, 2820–2822. [Google Scholar] [CrossRef]
- Al Bahri, M. Controlling domain wall thermal stability switching in magnetic nanowires for storage memory nanodevices. Journal of Magnetism and Magnetic Materials 2022, 543, 168611. [Google Scholar] [CrossRef]
- Ababei, R.V.; Ellis, M.O.A.; Vidamour, I.T.; Devadasan, D.S.; Allwood, D.A.; Vasilaki, E.; Hayward, T.J. Neuromorphic computation with a single magnetic domain wall. Scientific Reports 2021, 11, 15587. [Google Scholar] [CrossRef] [PubMed]
- Lequeux, S.; Sampaio, J.; Cros, V.; Yakushiji, K.; Fukushima, A.; Matsumoto, R.; Kubota, H.; Yuasa, S.; Grollier, J. A magnetic synapse: multilevel spin-torque memristor with perpendicular anisotropy. Scientific Reports 2016, 6, 31510. [Google Scholar] [CrossRef]
- Cubukcu, M.; Boulle, O.; Mikuszeit, N.; Hamelin, C.; Brächer, T.; Lamard, N.; Cyrille, M.C.; Buda-Prejbeanu, L.; Garello, K.; Miron, I.M.; et al. Ultra-Fast Perpendicular Spin-Orbit Torque MRAM. IEEE Transactions on Magnetics 2018, 54, 1–4. [Google Scholar] [CrossRef]
- Chen, J.Y.; DC, M.; Zhang, D.; Zhao, Z.; Li, M.; Wang, J.P. Field-free spin-orbit torque switching of composite perpendicular CoFeB/Gd/CoFeB layers utilized for three-terminal magnetic tunnel junctions. Applied Physics Letters 2017, 111, 012402. [Google Scholar] [CrossRef]
- Li, Z.; Shi, Y.; Chi, K.; Zhang, W.; Feng, X.; Xing, Y.; Meng, H.; Liu, B. Field-free spin-orbit torque induced magnetization reversal in a composite free layer with interlayer exchange coupling. Applied Physics Letters 2021, 118, 132402. [Google Scholar] [CrossRef]
- Lone, A.H.; Amara, S.; Fariborzi, H. Voltage-Controlled Domain Wall Motion-Based Neuron and Stochastic Magnetic Tunnel Junction Synapse for Neuromorphic Computing Applications. IEEE Journal on Exploratory Solid-State Computational Devices and Circuits 2022, 8, 1–9. [Google Scholar] [CrossRef]
- Liu, S.; Bennett, C.H.; Friedman, J.S.; Marinella, M.J.; Paydarfar, D.; Incorvia, J.A.C. Controllable Reset Behavior in Domain Wall-Magnetic Tunnel Junction Artificial Neurons for Task-Adaptable Computation. IEEE Magnetics Letters 2021, 12, 1–5. [Google Scholar] [CrossRef]
- Lone, A.H.; Li, H.; El-Atab, N.; Setti, G.; Fariborzi, H. Voltage-Gated Domain Wall Magnetic Tunnel Junction for Neuromorphic Computing Applications. IEEE Transactions on Electron Devices 2023, 70, 6293–6300. [Google Scholar] [CrossRef]
- Sengupta, A.; Roy, K. A Vision for All-Spin Neural Networks: A Device to System Perspective. IEEE Transactions on Circuits and Systems I: Regular Papers 2016, 63, 2267–2277. [Google Scholar] [CrossRef]
- Marrows, C.H.; Barker, J.; Moore, T.A.; Moorsom, T. Neuromorphic computing with spintronics. npj Spintronics 2024, 2, 12. [Google Scholar] [CrossRef]
- Heinze, S.; von Bergmann, K.; Menzel, M.; Brede, J.; Kubetzka, A.; Wiesendanger, R.; Bihlmayer, G.; Blügel, S. Spontaneous Atomic-Scale Magnetic Skyrmion Lattice in Two Dimensions. Nature Physics 2011, 7, 713–718. [Google Scholar] [CrossRef]
- Wu, Y. Magnetic whirlpools creep and flow in response to emergent electrodynamics. Nature 2024, 633, 527–528. [Google Scholar] [PubMed]
- Albert, F.; Reyren, N.; Cros, V. Magnetic skyrmions: Advances in physics and potential applications. Nature Reviews Materials 2017, 2. [Google Scholar] [CrossRef]
- Wu, Y.; Francisco, B.; Chen, Z.; Wang, W.; Zhang, Y.; Wan, C.; Han, X.; Chi, H.; Hou, Y.; Lodesani, A.; et al. A van der Waals interface hosting two groups of magnetic skyrmions. Advanced Materials 2022, 34, 2110583. [Google Scholar] [CrossRef] [PubMed]
- Mühlbauer, S.; Binz, B.; Jonietz, F.; Pfleiderer, C.; Rosch, A.; Neubauer, A.; Georgii, R.; Böni, P. Skyrmion Lattice in a Chiral Magnet. Science 2009, 323, 915–919. [Google Scholar] [CrossRef] [PubMed]
- Yu, X.; Kanazawa, N.; Onose, Y.; Kimoto, K.; Zhang, W.; Ishiwata, S.; Matsui, Y.; Tokura, Y. Near room-temperature formation of a skyrmion crystal in thin-films of the helimagnet FeGe. Nature Materials 2011, 10, 106–109. [Google Scholar] [CrossRef] [PubMed]
- Woo, S.; Litzius, K.; Krüger, B.; Im, M.Y.; Caretta, L.; Richter, K.; Mann, M.; Krone, A.; Reeve, R.; Weigand, M.; et al. Observation of room-temperature magnetic skyrmions and their current-driven dynamics in ultrathin metallic ferromagnets. Nature Materials 2016, 15. [Google Scholar] [CrossRef]
- Jiang, W.; Zhang, X.; Yu, G.; Zhang, W.; Wang, X.; Benjamin, J.M.; Pearson, J.E.; Cheng, X.; Heinonen, O.; Wang, K.L.; et al. Direct observation of the skyrmion Hall effect. Nature Physics 2016, 13, 162–169. [Google Scholar] [CrossRef]
- Tokunaga, Y.; Yu, X.Z.; White, J.S.; Rønnow, H.M.; Morikawa, D.; Taguchi, Y.; Tokura, Y. A new class of chiral materials hosting magnetic skyrmions beyond room temperature. Nature Communications 2015, 6. [Google Scholar] [CrossRef] [PubMed]
- Caretta, L.; Mann, M.; Büttner, F.; Ueda, K.; Pfau, B.; Günther, C.M.; Hessing, P.; Churikova, A.; Klose, C.; Schneider, M.; et al. Fast current-driven domain walls and small skyrmions in a compensated ferrimagnet. Nature nanotechnology 2018, 13, 1154–1160. [Google Scholar] [CrossRef] [PubMed]
- Mi, S.; Guo, J.; Hu, G.; Wang, G.; Li, S.; Gong, Z.; Jin, S.; Xu, R.; Pang, F.; Ji, W.; et al. Real-Space Topology-Engineering of Skyrmionic Spin Textures in a van der Waals Ferromagnet Fe3GaTe2. Nano Letters 2024, 24, 13094–13102. [Google Scholar] [CrossRef] [PubMed]
- Lone, A.H.; Ganguly, A.; Amara, S.; Das, G.; Fariborzi, H. Skyrmion-Magnetic Tunnel Junction Synapse With Long-Term and Short-Term Plasticity for Neuromorphic Computing. IEEE Transactions on Electron Devices 2022, 70, 371–378. [Google Scholar] [CrossRef]
- Yu, Z.; Shen, M.; Zeng, Z.; Liang, S.; Liu, Y.; Chen, M.L.; Zhang, Z.; Lu, Z.; You, L.; Yang, X.; et al. Voltage-controlled skyrmion-based nanodevices for neuromorphic computing using a synthetic antiferromagnet. Nanoscale Advances 2020, 2, 1309–1317. [Google Scholar] [CrossRef] [PubMed]
- Bindal, N.; Raj, R.K.; Rajib, M.M.; Atulasimha, J.; Kaushik, B.K. Antiferromagnetic Skyrmion based Energy-Efficient Leaky Integrate and Fire Neuron Device. Journal of Physics D: Applied Physics 2022. [Google Scholar] [CrossRef]
- Bindal, N.; Raj, R.K.; Kaushik, B.K. Antiferromagnetic skyrmion based shape-configured leaky-integrate-fire neuron device. Journal of Physics D: Applied Physics 2022, 55, 345007. [Google Scholar] [CrossRef]
- Lone, A.H.; Ganguly, A.; Li, H.; El-Atab, N.; Setti, G.; Das, G.; Fariborzi, H. Controlling the Skyrmion Density and Size for Quantized Convolutional Neural Network. IEEE Access 2023, 12, 149850–149860. [Google Scholar] [CrossRef]
- Yu, Z.; Shen, M.; Zeng, Z.; Liang, S.; Liu, Y.; Chen, M.L.; Zhang, Z.; Lu, Z.; Zhang, Y.; Xiong, R. Voltage-controlled skyrmion-based artificial synapse in a synthetic antiferromagnet. arXiv 2019, arXiv:1906.09758. [Google Scholar]
- Raab, K.; Brems, M.A.; Beneke, G.; Dohi, T.; Rothörl, J.; Kammerbauer, F.; Mentink, J.H.; Kläui, M. Brownian reservoir computing realized using geometrically confined skyrmion dynamics. Nature Communications 2022, 13, 6982. [Google Scholar] [CrossRef] [PubMed]
- Joksas, D.; AlMutairi, A.; Lee, O.; Cubukcu, M.; Lombardo, A.; Kurebayashi, H.; Kenyon, A.J.; Mehonic, A. Memristive, Spintronic, and 2D-Materials-Based Devices to Improve and Complement Computing Hardware. Advanced Intelligent Systems 2022, 4, 2200068. [Google Scholar] [CrossRef]
- Zhou, J.; Chen, J. Prospect of spintronics in neuromorphic computing. Advanced Electronic Materials 2021, 7, 2100465. [Google Scholar] [CrossRef]
- Ikeda, S.; Miura, K.; Yamamoto, H.; Mizunuma, K.; Gan, H.D.; Endo, M.; Kanai, S.; Hayakawa, J.; Matsukura, F.; Ohno, H. A perpendicular-anisotropy CoFeB–MgO magnetic tunnel junction. Nature Materials 2010, 9, 721–724. [Google Scholar] [CrossRef] [PubMed]
- Yuasa, S.; Djayaprawira, D.D. Giant tunnel magnetoresistance in magnetic tunnel junctions with a crystalline MgO(0 0 1) barrier. Journal of Physics D: Applied Physics 2007, 40, R337. [Google Scholar] [CrossRef]
- Miron, I.M.; Garello, K.; Gaudin, G.; Zermatten, P.J.; Costache, M.V.; Auffret, S.; Bandiera, S.; Rodmacq, B.; Schuhl, A.; Gambardella, P. Perpendicular switching of a single ferromagnetic layer induced by in-plane current injection. Nature 2011, 476, 189–193. [Google Scholar] [CrossRef] [PubMed]
- Khang, N.H.D.; Nakano, S.; Shirokura, T.; Miyamoto, Y.; Hai, P.N. Ultralow power spin–orbit torque magnetization switching induced by a non-epitaxial topological insulator on Si substrates. Scientific Reports 2020, 10, 12185. [Google Scholar] [CrossRef]
- Ghising, P.; Biswas, C.; Lee, Y.H. Graphene Spin Valves or Spin Logic Devices. Advanced Materials 2023, 35, 2209137. [Google Scholar] [CrossRef] [PubMed]
- Wang, C.P.; Cheng, S.H.; Hsueh, W.J. High spin current density in gate-tunable spin-valves based on graphene nanoribbons. Scientific Reports 2023, 13, 9234. [Google Scholar] [CrossRef] [PubMed]
- Jiang, W.; Upadhyaya, P.; Zhang, W.; Yu, G.; Jungfleisch, M.B.; Fradin, F.Y.; Pearson, J.E.; Tserkovnyak, Y.; Wang, K.L.; Heinonen, O.; et al. Blowing magnetic skyrmion bubbles. Science 2015, 349, 283–286. [Google Scholar] [CrossRef] [PubMed]
- Tang, J.; He, C.; Tang, J.; Yue, K.; Zhang, Q.; Liu, Y.; Wang, Q.; Wang, S.; Li, N.; Shen, C.; et al. A Reliable All-2D Materials Artificial Synapse for High Energy-Efficient Neuromorphic Computing. Advanced Functional Materials 2021, 31, 2011083. [Google Scholar] [CrossRef]
- Kim, S.; Choi, S.; Lee, H.G.; Jin, D.; Kim, G.; Kim, T.; Lee, J.S.; Shim, W. Neuromorphic van der Waals crystals for substantial energy generation. Nature Communications 2021, 12, 47. [Google Scholar] [CrossRef]
- Sun, Y.; Li, M.; Ding, Y.; Wang, H.; Wang, H.; Chen, Z.; Xie, D. Programmable van-der-Waals heterostructure-enabled optoelectronic synaptic floating-gate transistors with ultra-low energy consumption. InfoMat 2022, 4, e12317. [Google Scholar] [CrossRef]
- Grollier, J.; Querlioz, D.; Camsari, K.Y.; Everschor-Sitte, K.; Fukami, S.; Stiles, M.D. Neuromorphic spintronics. Nature Electronics 2019, 3, 360–370. [Google Scholar] [CrossRef]
- Joksas, D.; AlMutairi, A.; Lee, O.; Cubukcu, M.; Lombardo, A.; Kurebayashi, H.; Kenyon, A.J.; Mehonic, A. Memristive, Spintronic, and 2D-Materials-Based Devices to Improve and Complement Computing Hardware. Advanced Intelligent Systems 2022, 4, 2200068. [Google Scholar] [CrossRef]
- Zabihi, M.; Chowdhury, Z.I.; Zhao, Z.; Karpuzcu, U.R.; Wang, J.P.; Sapatnekar, S.S. In-Memory Processing on the Spintronic CRAM: From Hardware Design to Application Mapping. IEEE Transactions on Computers 2019, 68, 1159–1174. [Google Scholar] [CrossRef]
- Shumilin, A.; Neha, P.; Benini, M.; Rakshit, R.; Singh, M.; Graziosi, P.; Cecchini, R.; Gnoli, L.; Prezioso, M.; Bergenti, I.; et al. Glassy Synaptic Time Dynamics in Molecular La0.7Sr0.3MnO3/Gaq3/AlOx/Co Spintronic Crossbar Devices. Advanced Electronic Materials 2024, 10, 2300887. [Google Scholar] [CrossRef]
- Kumari, S.; Pradhan, D.K.; Pradhan, N.R.; Rack, P.D. Recent developments on 2D magnetic materials: challenges and opportunities. Emergent Materials 2021, 4, 827–846. [Google Scholar] [CrossRef]
- Lin, Z.; Peng, Y.; Wu, B.; Wang, C.; Luo, Z.; Yang, J. Magnetic van der Waals materials: Synthesis, structure, magnetism, and their potential applications. Chinese Physics B 2022, 31, 087506. [Google Scholar] [CrossRef]
- Hao, Q.; Dai, H.; Cai, M.; Chen, X.; Xing, Y.; Chen, H.; Zhai, T.; Wang, X.; Han, J.B. 2D Magnetic Heterostructures and Emergent Spintronic Devices. Advanced Electronic Materials 2022, 8, 2200164. [Google Scholar] [CrossRef]
- Ansari, M.S.; Othman, M.H.D.; Ansari, M.O.; et al. Progress in Fe3O4-centered spintronic systems: Development, architecture, and features. Applied Materials Today 2021, 25, 101181. [Google Scholar] [CrossRef]
- Dieny, B.; Prejbeanu, I.L.; Garello, K.; Gambardella, P.; Freitas, P.; Lehndorff, R.; Raberg, W.; Ebels, U.; Demokritov, S.O.; Akerman, J.; et al. Opportunities and challenges for spintronics in the microelectronics industry. Nature Electronics 2020, 3, 446–459. [Google Scholar] [CrossRef]




| Device | Efficiency | Scalability | Temp. (K) | Switch Speed | Footprint | Leakage | Error Rate | Refs. |
|---|---|---|---|---|---|---|---|---|
| MTJ | 10–100 fJ/bit | >1 Tb/in2 | 300 | 1–10 ns | 20–50 nm | NA | 10−5 | [87,88] |
| SOT Devices | 10–20 fJ/bit | Sub 10 nm | 300 | <1 ns | <50 nm | NA | 10−5 | [89,90] |
| Spin Valves | 10−16J/event | 10 nm | 300 | <10 ns | 50 nm | NA | 10−4 | [91,92] |
| Skyrmions | 0.3-1 fJ/event | Sub 100 nm | 300 | 100 m/s | <100 nm | NA | 10−3 | [69,93] |
| vdW HS | 2.5 fJ/event | ∼10nm | 300 | ∼40 ns | <10 nm | NA | 10−2 | [8,94,95] |
Disclaimer/Publisher’s Note: The statements, opinions and data contained in all publications are solely those of the individual author(s) and contributor(s) and not of MDPI and/or the editor(s). MDPI and/or the editor(s) disclaim responsibility for any injury to people or property resulting from any ideas, methods, instructions or products referred to in the content. |
© 2025 by the authors. Licensee MDPI, Basel, Switzerland. This article is an open access article distributed under the terms and conditions of the Creative Commons Attribution (CC BY) license (http://creativecommons.org/licenses/by/4.0/).