Preprint Article Version 1 Preserved in Portico This version is not peer-reviewed

Optimization of a Low-cost Corona-DBD Plasma Wastewater Treatment System through CCD/RSM with Mechanistic and Efficiency Analysis

Version 1 : Received: 10 December 2023 / Approved: 11 December 2023 / Online: 11 December 2023 (16:38:11 CET)

A peer-reviewed article of this Preprint also exists.

Xiao, Y.; Tian, Y.; Zhan, Y.; Zhu, J. Optimization of a Low-Cost Corona Dielectric-Barrier Discharge Plasma Wastewater Treatment System through Central Composite Design/Response Surface Methodology with Mechanistic and Efficiency Analysis. Sustainability 2024, 16, 605. Xiao, Y.; Tian, Y.; Zhan, Y.; Zhu, J. Optimization of a Low-Cost Corona Dielectric-Barrier Discharge Plasma Wastewater Treatment System through Central Composite Design/Response Surface Methodology with Mechanistic and Efficiency Analysis. Sustainability 2024, 16, 605.

Abstract

Water pollution, intensified by the release of hard-to-degrade pollutants, poses severe threats to ecosystems, human health, and economic development. The existing advanced oxidation processes often involve high operational costs and may result in secondary pollution, highlighting the necessity for innovative and more sustainable solutions. To address these challenges, our study introduces a cost-effective and eco-friendly corona discharge barrier plasma discharger for wastewater treatment. Through the central composite design/response surface methodology, a high decolorization rate of 98% of methylene blue (MB) within 10 minutes was achieved by optimizing parameters such as pH and voltage. Furthermore, the mechanisms of the generation of reactive oxygen species via this device was discussed in detail and the degradation pathways of MB were described. Moreover, this device is also very energy-efficient, with a low energy density and electrical energy per order of 0.15 watt/mL and 5.79 kWh/m³/order, respectively. In conclusion, the plasma discharger developed in this study provides a cost-effective and environmentally sustainable solution for dye wastewater treatment. This research contributes significantly to the advancement of sustainable dye wastewater management practices, offering an innovative method that meets both environmental and economic objectives.

Keywords

Water purification; non-thermal plasma; reactor design; advanced purification systems

Subject

Environmental and Earth Sciences, Pollution

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