Preprint Article Version 1 Preserved in Portico This version is not peer-reviewed

Enhanced Performances of Quantum Dot Light-Emitting Diodes with an Organic–Inorganic Hybrid Hole Injection Layer

Version 1 : Received: 5 June 2023 / Approved: 6 June 2023 / Online: 6 June 2023 (08:08:58 CEST)

A peer-reviewed article of this Preprint also exists.

Chen, L.; Jiang, D.; Du, W.; Shang, J.; Li, D.; Liu, S. Enhanced Performances of Quantum Dot Light-Emitting Diodes with an Organic–Inorganic Hybrid Hole Injection Layer. Crystals 2023, 13, 966. Chen, L.; Jiang, D.; Du, W.; Shang, J.; Li, D.; Liu, S. Enhanced Performances of Quantum Dot Light-Emitting Diodes with an Organic–Inorganic Hybrid Hole Injection Layer. Crystals 2023, 13, 966.

Abstract

PEDOT:PSS (polyethylene dioxythiophene:polystyrenesulfonate) is a commonly used hole injec-tion layer (HIL) in optoelectronic devices due to its high conductive properties and work function. However, the acidic and hygroscopic nature of PEDOT:PSS can be problematic for device stability over time. To address this issue, in this study, we have demonstrated the potential of an organic-inorganic hybrid HIL, by incorporating solution-processed WOx nanoparticles (WOx NPs) into the PEDOT:PSS mixture. This hybrid solution was found to have a superior hole transport ability and low Ohmic contact resistance, contributing to higher brightness (~62 000 cd m-2) and current efficiency (13.1 cd A-1) in the manufactured quantum-dot based light-emitting diodes (QLEDs). In addition, the resulting devices achieved a relative operational lifetime of 7,071 hours, or approxi-mately twice that of traditional QLEDs with PEDOT:PSS HILs. The proposed method is an un-complicated, reliable and low-cost way to achieve long operational lifetimes without sacrificing efficiency in optoelectronic devices.

Keywords

WOx nanoparticle doped PEDOT:PSS; hole injection layer; quantum dot; light-emitting diode

Subject

Physical Sciences, Quantum Science and Technology

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