Preprint Article Version 1 Preserved in Portico This version is not peer-reviewed

Thoron gas measurement using an airflow-through scintillation cell with consideration for progeny deposition

Version 1 : Received: 27 March 2023 / Approved: 28 March 2023 / Online: 28 March 2023 (02:49:17 CEST)

A peer-reviewed article of this Preprint also exists.

Zhao, C.; Liu, J.; Chen, Y.; He, L.; Tang, F.; Zhuo, W. Thoron Gas Measurement Using Airflow-Through Scintillation Cell with Consideration of Progeny Deposition. Atmosphere 2023, 14, 831. Zhao, C.; Liu, J.; Chen, Y.; He, L.; Tang, F.; Zhuo, W. Thoron Gas Measurement Using Airflow-Through Scintillation Cell with Consideration of Progeny Deposition. Atmosphere 2023, 14, 831.

Abstract

Accurate measurement of low-level thoron gas and high-accuracy calibration of thoron measurement devices are essential for assessing and preventing thoron radiological risks. This study aimed to develop a thoron gas measurement technique using an airflow-through scintillation cell for both low-level measurement and high-accuracy calibration. To achieve this, a compartment model was developed to estimate the influence of progeny deposition and accumulation on the wall of the scintillation cell to prevent overestimation of thoron. A self-developed scintillation cell was utilized to implement and validate this technique. The lower detection limit and measurement uncertainty were then evaluated to assess the feasibility of the technique for low-level measurement and high-accuracy calibration. The results showed that the compartment model effectively addressed the influence of the progeny deposition. The measurement technique achieved a lower detection limit below 100 Bq m-3 even with the coexistence of 100 Bq m-3 of radon and attained a measurement uncertainty (k = 2) below 10% when the concentration of thoron exceeded 1,000 Bq m-3. In summary, this study developed a reliable and practical thoron gas measurement technique using an airflow-through scintillation cell with consideration for progeny deposition, and is expected to contribute to the assessment and prevention of thoron radiological risk.

Keywords

thoron measurement; airflow-through scintillation cell; progeny accumulation effect; compartment model; low-level measurement; calibration

Subject

Physical Sciences, Fluids and Plasmas Physics

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